Select the most appropriate direct form of the given sentence.

She demanded of her younger brother why he had taken her paints without her permission.

1
She said to her younger brother angrily, “Why do you take my paints without my permission?”
2
She asked her younger brother angrily, “Why do you have to take my paints without my permission?”
3
She said to her younger brother angrily, “Why have you taken my paints without my permission?”
4
She said to her younger brother, “Why he had taken her paints without her permission?”

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